Source: MICHIGAN STATE UNIV submitted to NRP
THE ROLE OF LIPOLYSIS PRODUCTS IN THE MODULATION OF ADIPOSE TISSUE METABOLIC FUNCTION IN PERIPARTURIENT DAIRY COWS DURING HEALTH AND DISEASE
Sponsoring Institution
National Institute of Food and Agriculture
Project Status
ACTIVE
Funding Source
Reporting Frequency
Annual
Accession No.
1025473
Grant No.
(N/A)
Cumulative Award Amt.
(N/A)
Proposal No.
(N/A)
Multistate No.
(N/A)
Project Start Date
Apr 1, 2021
Project End Date
Mar 31, 2026
Grant Year
(N/A)
Program Code
[(N/A)]- (N/A)
Recipient Organization
MICHIGAN STATE UNIV
(N/A)
EAST LANSING,MI 48824
Performing Department
Large Animal Clinical Sciences
Non Technical Summary
During the periparturient period of dairy cows, adipose tissues (AT) lipolysis fulfills, in part, energy deficits driven by fetal growth and the onset of lactation. Lipolysis induces a remodeling process within AT that is characterized by a moderate inflammatory response with infiltration of macrophages. In periparturient cows that successfully transition into lactation, lipolysis rate decreases and AT inflammation resolves as lactation progresses. However, when lipolysis rate is not reduced, AT inflammation is maintained leading to poor lactation performance and to metabolic and infectious diseases. To make things more complicated, periparturient illnesses occur as complexes that pose severe welfare issues to dairy cows. During lipolysis adipocytes produce hydroxyl-octadecadienoic acids (HODEs) from linoleic acid through enzymatic and non-enzymatic reactions. These lipolytic products are potent modulators of inflammatory responses in AT that may directly increase lipolysis rate by reducing adipocyte response to insulin. An additional periparturient factor that is strongly connected with the presentation of disease complexes is the sharp increase in circulating bacterial endotoxins. Our central hypothesis is that lipolysis dysregulation increases the abundance of a select group of HODEs in AT in a non-enzymatic, ROS dependent manner. This increase enhances ATM infiltration and sustains AT inflammation and this response is exacerbated during exposure to endotoxins. We will test this hypothesis using in vitro and ex-vivo models of AT lipolysis, and in periparturient cows using a nutritional intervention for lipolysis modulation. We will pursue three objectives 1:Determine how HODEs that are synthesized in bovine AT during lipolysis modify the macrophage phenotype and reduce the anti-lipolytic response of adipocytes to insulin. 2: Determine how endotoxins enhance adipocytes' lipolytic responses. Our working hypothesis is that endotoxins trigger lipolysis dysregulation through changes in adipocytes' insulin sensitivity and ATM phenotype. 3: Determine how inhibiting lipolysis in periparturient dairy cows affects the non-enzymatic biosynthesis and profile of HODEs, and the ATM phenotype. Upon completion of this project, we will be able to determine the role of HODEs in the vicious cycle of lipolysis dysregulation and chronic inflammation in AT. These findings will support their use as diagnostic, nutritional, or pharmacological targets in management programs of periparturient dairy cows. In addition, this project will elucidate the mechanisms by which endotoxemia induces lipolysis dysregulation and increases periparturient dairy cows' susceptibility to diseases. Our long-term goal is to develop nutritional and pharmacological tools to prevent lipolysis dysregulation during periods of NEB. We expect these tools will benefit herd health, improve dairy cows' welfare, and increase the economic sustainability of dairy farming.
Animal Health Component
50%
Research Effort Categories
Basic
50%
Applied
50%
Developmental
(N/A)
Classification

Knowledge Area (KA)Subject of Investigation (SOI)Field of Science (FOS)Percent
3113410106050%
3083410101050%
Goals / Objectives
In this project, we propose that lipolysis dysregulation and abnormal AT inflammation, including macrophage infiltration and polarization, become connected through the actions of the lipolysis derived linoleic acid metabolites called HODEs (hydroxyl-octadecadienoic acids) and are excacerbated by endotoxin exposure. HODEs are highly bioactive oxylipids that are synthesized enzymatically and nonenzymatically from the linoleic acid released during lipolysis [59]. Our previous research strongly indicate that A) lipolysis is associated with plasma and AT content of HODEs and their substrate, linoleic acid; and B) HODEs are powerful modulators of macrophages' inflammatory phenotype.Our central hypothesis is that lipolysis dysregulation increases the abundance of a select group of HODEs in AT in a non-enzymatic, ROS dependent manner. This increase enhances ATM infiltration and sustains AT inflammation and this response is excacerbated during exposure to endotoxins. We will test this hypothesis using in vitro and ex-vivo models of AT lipolysis, and in periparturient cows using a nutritional intervention for lipolysis modulation. We will pursue three objectives:bjective 1:Determine how HODEs that are synthesized in bovine AT during lipolysis modify the macrophage phenotype and reduce the anti-lipolytic response of adipocytes to insulin.Objective 2: Determine how endotoxins enhance adipocytes' lipolytic responses. Our working hypothesis is that endotoxins trigger lipolysis dysregulation through changes in adipocytes' insulin sensitivity and ATM phenotype.Objective 3: Determine how inhibiting lipolysis in periparturient dairy cows affects the non-enzymatic biosynthesis and profile of HODEs, and the ATM phenotype.
Project Methods
Objective 1: Experiment 1A1: How does hormone-sensitive lipase (HSL) activity affect HODE biosynthesis in adipocytes?We will stimulate differentiated primary adipocytes with 10 µM of isoproterenol (ISO) to induce lipolysis [0 µM as control (CON)]. After 4 h, we will harvest adipocytes and culture media and quantify FA, HODEs, and other lipid mediators of inflammation by high-performance liquid chromatography-mass spectrometry (HPLC-MS/MS). To further characterize how lipolysis affects adipocyte inflammatory responses, we will evaluate the expression profiles of pro-inflammatory cytokines and enzymes involved in either synthesizing oxylipids or FA metabolism using RT-qPCR, protein blotting, and ELISA. We will evaluate cell viability both before and after treatments. To determine the direct effect of HSL activation on HODE biosynthesis, we will use an inhibitor of HSL [CAY10499, or NIA, niacin 2µM] during the lipolytic stimulus. For this experiment, adipocytes will be exposed to CAY10499 [10 µM] or NIA for 1 h before ISO stimulation. After 4 hours of ISO exposure, we will harvest the adipocytes and media and assess each lipolytic and inflammatory variables.Experiment 1A2. How does HSL activity affect the non-enzymatic biosynthesis of HODEs by ROS-mediated oxidation?We will expose differentiated primary adipocytes to CON or ISO as described above in Experiment 1A1. To determine how ROS, 15LOX, and COX2 affect HODEs biosynthesis during lipolysis, we will treat adipocytes with the following inhibitors: a) a 15LOX inhibitor (PD146176, 2µM); b) a COX2 inhibitor (celecoxib, 5µM); c) an inhibitor of the nicotinamide adenine dinucleotide phosphate oxidase that minimizes ROS production (diphenyliodonium (DPI), 10 µM); d) PD146176+celecoxib, e) PD146176+DPI, f) PD146176+celecoxib+DPI, g) celecoxib+DPI h) a negative control treatment; and i) a positive oxidative control [H2O2, 200 µM]. We will evaluate cell viability both before and after treatments, and collect cells and media as described in experiment 1A1 for HODEs detection and quantification, and gene and protein profiling. We will assess the generation of ROS in adipocytes using: a) the OxiSelect intracellular detection assay, and b) quantifying isoprostanes as a proxy of oxidative stress status.Experiment 1B1. How do HODEs affect markers of bovine macrophage phenotype?We will harvest myeloid-derived monocytes from blood by Ficoll gradient. After they mature into macrophages (M0), we will expose the cells to different concentrations of 9-, 10-, 12-, and 13- HODEs for 24 h (0, 5, 10 and 50 nmol). The doses we selected are based on the plasma concentrations of HODEs that we detected in periparturient cows in our preliminary studies. We will polarize primary bovine macrophages to either the M1 or M2 phenotype for use as positive controls. We will use non-stimulated (M0) macrophages as negative phenotypic controls.Experiment 1B2. What is the direct effect of HODEs on the anti-lipolytic response of adipocytes to insulin?We will expose adipocytes to different concentrations of HODEs for 1 h, and then stimulate lipolysis with 10 μM of ISO with or without insulin (0.2 μg/L). We will test the potency of insulin's anti-lipolytic effect in the adipocytes by measuring a) FA uptake (without ISO stimulation), b) NEFA and glycerol release, c) the expression of genes in the insulin signaling network, and d) the expression/phosphorylation of lipolysis and insulin signaling proteins. We will focus on measuring PKA activity because this kinase phosphorylates HSL, which activates it and induces its translocation to the lipid droplet. It has been suggested that PKA activity is not effectively controlled during lipolysis dysregulation, which could exacerbate the release of NEFA.Objective 2. Determine how endotoxins enhance adipocytes' lipolytic responsesExperiment 2A1 TLR2 and TLR4 activation by LPS and LTA induces lipolysis in bovine adipocytes:We will differentiate primary preadipocytes to adipocytes for 10 d. Then, we will treat the adipocytes for 72h with non-targeting siRNA (Nsp) pools or siRNA ON-TARGET Plus SMARTpool siRNAs targeting TLR2 , TLR4, or both TLR2 and TLR4 according to manufacturer's instructions and using FuGENE transfection reagent. We will optimize the concentration of siRNA prior to the experiments with endotoxin. We will validate TLR2, TLR4, and TLR2/4 knockdown by real-time PCR and western blotting. For all siRNA experiments, cell-viability will be determined with the LIVE/DEAD viability kit. Next, we will treat the adipocytes, including un-transfected and transfection reagent controls, with 1 μM of ISO to induce lipolysis [0 μM as a basal control (BAS)] in the presence or absence of LPS (O55:B5, 20µg/ml) and LTA (Staph aureus 50µg/ml) for 7 h. Thereafter, we will harvest the adipocytes and collect the culture media. We will quantify lipolysis by measuring FFA and glycerol release. We will use an inhibitor of HSL, CAY10499 (10 μM), as a positive control for total inhibition of lipolysis.We will evaluate these two metabolic processes using a systems biology approach. 1) At the transcriptomic level we will use RT-qPCR to determine the effect of endotoxin on gene markers of inflammation, lipogenesis, lipolysis, and insulin signaling. We will perform transcriptomics analyses as described by our group. 2) Certain components of lipolysis and of the inflammatory pathways induced by endotoxin are controlled post-transcriptionally and must be evaluated at the protein level. Therefore, it is necessary to determine not only the protein content, but also the phosphorylation levels of specific peptides that are markers of lipolysis and insulin sensitivity in AT. We will quantify these proteins using traditional western blotting and capillary electrophoresis. 3) Since endotoxins are potent inflammation inducers and lipolysis is an inflammatory event, we will perform a detailed characterization of the chemokine and cytokine profiles of adipocytes and ATM.Experiment 2A2 TLR2 and TLR-4 activation by LPS and LTA trigger the classic and inflammatory lipolytic pathways in bovine adipocytes: To determine how LPS and LTA affect lipolysis, we will use inhibitors to block the following steps of the classical and inflammatory lipolytic pathways: 1) PKA: H-89 (20 µM), 2) PKC: Ro-31-8220 (1 µM), 3) ERK 1/2 : U0126 (2 µM), 4) NFκB: PDTC (80 µM), and 5) TNF-α: CAS 1049741 (22 µM). We will pre-incubate un-transfected, Nsp, and siRNA treated adipocytes with the inhibitors for 1h, and then induce lipolysis with ISO, LPS, and LTA. We will use inhibitors alone (without lipolysis treatment) as negative controls. After 7 h, we will harvest the adipocytes and collect the culture media [90]. We will quantify lipolysis by measuring FFA and glycerol release.Aim 3. Determine how inhibiting lipolysis in periparturient dairy cows affects the biosynthesis and profile of HODEs, ATM phenotype, and AT response to insulin.Experimental Design. All procedures will be approved by the MSU Institutional Animal Care and Use Committee. We will select 40 gestating non-lactating multiparous Holstein cows from the MSU Dairy Field Laboratory 1 week after dry-off. The inclusion criteria are 1) pregnant, 2) 210 to 230 days of gestation, and 3) BCS between 3.25 and 3.75. Cows will be blocked by parity and BCS and then randomly assigned at close-up (d-21) to either the NIA (12g/d NiaShure™) or control (CON) group. At 12 g/d, rumen-protected NIA decreases lipolysis induced by negative energy balance. From dry-off and until ~21 d before expected calving, cows will receive a common dry cow diet. A close-up diet will be fed starting day -21 before expected calving. Cows will move onto a fresh cow diet at calving, and will continue receiving NIA (12g/d) or no NIA (CON) until 21 days after calving

Progress 04/01/21 to 09/30/21

Outputs
Target Audience:Nutritionists, veterinarians, animal scientists, professional students (veterinary medicine), veterinary technicians, and undergraduate students (animal sciences and physiology). Changes/Problems:The in vitro experiments planned for all aims have beend delayed due to serious issues with backordering of tissue culture supplies due to supply chain disruptions. For examples 96 well plates and glycerol reagent were backordered for nearly 7 months during 2021. Without these supplies we could not advance in our mechanistic experiments What opportunities for training and professional development has the project provided?The following persons are being trained as part of this project: 1. Madison Smith, DVM/PhD student 2. Ursula Abou-Rjeileh. PhD student 3. Miguel Chirivi. PhD student 4. Jair Parales. PhD student How have the results been disseminated to communities of interest?Knowledge generated by this project was disseminated through peer-reviewed publications in high impact factor journals and by presenting findings in regional, national, and international conferences where graduate students and the PIs participated. We also prepared one lay article that was published in MSU extension https://www.canr.msu.edu/news/harnessing-fatty-acids-for-transition-cow-management What do you plan to do during the next reporting period to accomplish the goals?All aims currently have samples collected that are being processed. During 2022 the results will be consolidated and knwoledge will be diseminated in regional, national, and international meetings.

Impacts
What was accomplished under these goals? 1. In objective 1: Based on our published data demonstrating the HODEs are synthesized during lipolysisis, we are currently characterizing how the production of these oxylipids alters the expression of gene networks that reflect macrophage phenotype profile and adipocyte sensitivity to insulin. In 2020 we published an RNAseq study that identified some of these markers (PBMC7686742). Now we are using those markers to evaluate the effect of diets that reduce periparrturient lipolysis 2. In objective 2: We determined that endotoxins induce lipolysis through 2 specific pathways, the classical and the inflammatory. At the same time, the inflammatory responses impair adipocytes' response to insulin (PMID 34696909). 3. In objective 3: We completed a feeding trial that used chromium and palmitic acid in periparturient cows as a way to reduce lipolysis around parturition. We are currently evaluating the effects on HODEs

Publications

  • Type: Journal Articles Status: Published Year Published: 2021 Citation: Abou-Rjeileh U, Contreras GA. Redox Regulation of Lipid Mobilization in Adipose Tissues. Antioxidants (Basel). 2021 Jul 7;10(7). doi: 10.3390/antiox10071090. Review. PubMed PMID: 34356323; PubMed Central PMCID: PMC8301038
  • Type: Conference Papers and Presentations Status: Published Year Published: 2021 Citation: Abou-Rjeileh U, Lock AL, Contreras GA. The effect of palmitic and oleic acids on lipogenesis in dairy cow adipocytes. 2021 Tri-State Dairy Nutrition Conference. Apr 19-21, pp 164. 1st place MS student competition.
  • Type: Conference Papers and Presentations Status: Published Year Published: 2021 Citation: Chirivi M, Rendon C, Myers M, Contreras GA. Lipopolysaccharide induces lipolysis and insulin resistance in adipose tissue from dairy cows. 2021 Tri-State Dairy Nutrition Conference, Apr 19-21. pp 166.
  • Type: Conference Papers and Presentations Status: Published Year Published: 2021 Citation: Myers MN, Rendon CJ, Zachut M, Tam J, Contreras GA. Cannabinoids modulate adipogenesis and lipogenesis in dairy cows. International Cannabinoid Research Society Annual Meeting. June 21-24, 2021, Jerusalem, Israel. Pp 167
  • Type: Conference Papers and Presentations Status: Published Year Published: 2021 Citation: Myers MN, Rendon CJ, Zachut M, Tam J, Contreras GA. Adipogenesis and lipogenesis are modulated by cannabinoids in dairy cows. American Dairy Science Association Annual Meeting, July 11-14, 2021, SC138
  • Type: Journal Articles Status: Published Year Published: 2021 Citation: Chirivi M, Rendon CJ, Myers MN, Prom CM, Roy S, Sen A, Lock AL, Contreras GA. Lipopolysaccharide induces lipolysis and insulin resistance in adipose tissue from dairy cows. J Dairy Sci. 2022 Jan;105(1):842-855. doi: 10.3168/jds.2021- 20855. Epub 2021 Oct 23. PubMed PMID: 34696909.
  • Type: Journal Articles Status: Published Year Published: 2021 Citation: Zachut M, Contreras GA. Symposium review: Mechanistic insights into adipose tissue inflammation and oxidative stress in periparturient dairy cows. J Dairy Sci. 2022 Feb 9;. doi: 10.3168/jds.2021-21225. [Epub ahead of print] Review. PubMed PMID: 35151484.
  • Type: Journal Articles Status: Published Year Published: 2022 Citation: Putman AK, Gandy JC, Contreras GA, Sordillo LM. Oxylipids are associated with higher disease risk in postpartum cows. J Dairy Sci. 2022 Mar;105(3):2531-2543. doi: 10.3168/jds.2021-21057. Epub 2022 Jan 25. PubMed PMID: 35086706
  • Type: Conference Papers and Presentations Status: Published Year Published: 2021 Citation: Abou-Rjeileh U, Lock AL, Contreras GA. Palmitic and oleic acids modulate lipogenesis in dairy cow adipocytes. American Dairy Science Association Annual Meeting, July 11-14, 2021, 264
  • Type: Conference Papers and Presentations Status: Published Year Published: 2021 Citation: Abou-Rjeileh U, Chirivi M, Giron JP, Lock AL, Zachut M, Tam J, Contreras GA. Cannabinoids and adipose tissue lipolysis in periparturient dairy cows. American Dairy Science Association Annual Meeting, July 11-14, 2021 284
  • Type: Conference Papers and Presentations Status: Published Year Published: 2021 Citation: Abou-Rjeileh U, Chirivi M, Parales-Giron J, Dos Santos Neto JM, Prom CM, Laguna J, Lock AL, Contreras GA. Oleic acid improves insulin sensitivity in adipose tissue of periparturient dairy cows. Phi Zeta Research Day, Michigan State University. October 1st 2021. pp13 1st place graduate student competition oral presentation
  • Type: Conference Papers and Presentations Status: Published Year Published: 2021 Citation: Chirivi M, Contreras GA. Endotoxin Activates Lipolysis in Bovine Adipocytes. Phi Zeta Research Day, Michigan State University. October 1st 2021. pp15
  • Type: Conference Papers and Presentations Status: Published Year Published: 2021 Citation: Cortes D, Chirivi M, OConnor A, Contreras GA. Lipolysis Inhibition Improves Clinical Outcomes In The Treatment Of Ketosis In Dairy Cows. Phi Zeta Research Day, Michigan State University. October 1st 2021. pp15
  • Type: Conference Papers and Presentations Status: Published Year Published: 2021 Citation: Myers M, Chirivi M, Abou-Rjeileh U, Zachut M, Tam J, Contreras GA. Adipose Tissue Adipogenesis and Lipogenesis Are Modulated by Cannabinoids in Dairy Cows. Phi Zeta Research Day, Michigan State University. October 1st 2021. pp19 1st place graduate student competition poster presentation.
  • Type: Conference Papers and Presentations Status: Published Year Published: 2021 Citation: Abou-Rjeileh U, Chirivi M, Parales-Giron J, Prom CM, Laguna J, Lock AL, Contreras GA. Oleic acid improves insulin sensitivity in dairy cow adipose tissue through PPAR? and PLIN5. CRWAD 2021, December 5-7, Chicago, IL. Pp 33. Travel award recipient.
  • Type: Conference Papers and Presentations Status: Published Year Published: 2021 Citation: Contreras GA. Oxidative stress in the adipose tissue: Magnifying the risk for periparturient disease. Animal Health Symposium: Adipose Tissue in Transition Dairy Cows as an Integrator of Metabolic and Inflammatory Cues in Health and Disease. American Dairy Science Association Annual Meeting, July 11-14, 2021, S121
  • Type: Conference Papers and Presentations Status: Published Year Published: 2021 Citation: Contreras GA, Putman A, Abuelo A, Sordillo LM. Lactational Biology Symposium: Metabolic transitions and lipid mediators as modulators of mammary gland inflammation and oxidative stress. American Dairy Science Association Annual Meeting 2021, Fall Seminars, W112.