Source: UNIVERSITY OF CALIFORNIA, DAVIS submitted to NRP
TACKLING THE LOW EFFICIENCY OF PROTEIN PRODUCTION BY RUMEN MICROBES: A CELLULAR AND WHOLE-ANIMAL APPROACH
Sponsoring Institution
National Institute of Food and Agriculture
Project Status
ACTIVE
Funding Source
Reporting Frequency
Annual
Accession No.
1023959
Grant No.
2018-67015-32517
Cumulative Award Amt.
$500,000.00
Proposal No.
2018-09548
Multistate No.
(N/A)
Project Start Date
Apr 1, 2019
Project End Date
Mar 31, 2026
Grant Year
2020
Program Code
[A1231]- Animal Health and Production and Animal Products: Improved Nutritional Performance, Growth, and Lactation of Animals
Recipient Organization
UNIVERSITY OF CALIFORNIA, DAVIS
410 MRAK HALL
DAVIS,CA 95616-8671
Performing Department
Animal Science
Non Technical Summary
Ruminants (cows, sheep, goats) are unique because most of the protein they digest comes from microbes growing in the forestomach (rumen). Increasing this microbial protein is a perennial goal of ruminant nutrition, but progress has stalled because microbes grow with poor efficiency and for reasons that are unclear. In fact, we do not know how inefficient microbes really are; it is uncertain how much cellular energy (ATP) they generate during metabolism and have available for growth. Our overarching hypothesis is that microbes grow with poor efficiency because they direct ATP energy away from growth and towards energy sinks. We further hypothesize that microbes generate more ATP energy during metabolism than previously realized, and thus they grow with even poorer efficiency than thought. To test these hypotheses, we propose the specific aims of 1) determining how much ATP energy microbes expend on two energy sinks (maintenance and glycogen synthesis) 2) determining how much ATP energy cells yield during metabolism of carbohydrate (glucose). We will use experiments spanning from laboratory cultures of bacteria to dairy cows, and we expect our results to show both energy sinks (maintenance, glycogen synthesis) are large and important to decreasing efficiency. However, we expect the exact importance of each sink varies with the animal diet and microbial group. We further expect our results to show that microbes generate up to 50% more ATP energy during metabolism of glucose than previously recognized. We anticipate the impact of this project will be to reveal mechanisms behind poor growth efficiency, guide strategies to increase microbial efficiency, and reduce feeding of protein to ruminants. We anticipate that we could improve efficiency by at least 5%, reducing feed costs for the US dairy industry by $122 million/yr.
Animal Health Component
10%
Research Effort Categories
Basic
90%
Applied
10%
Developmental
(N/A)
Classification

Knowledge Area (KA)Subject of Investigation (SOI)Field of Science (FOS)Percent
3023410101050%
3023410110050%
Goals / Objectives
Objective 1. Determine how much ATP that mixed rumen bacteria expend on maintenance when provided differentcarbohydrates (glucose, starch, fiber).Objective 2. Determine how much ATP that mixed rumen microbes expend on glycogen synthesis in vivo.Objective 3. Determine the ATP yield from the major fermentation pathways of glucose (hexose).
Project Methods
Aim 1.Determine how much ATP that mixed rumen bacteria expend on maintenance when provided different carbohydrates (glucose, starch, fiber).Study 1 (Mixed bacteria)We will inoculate a system of continuous-culture fermenters with rumen contents from four lactating cows fed a corn silage based diet. To maintain bacteria at different growth rates, fermenters will be maintained at a range of dilution rates (2.0, 6.0, 8.0, 12.0/% h) by adjusting rate of buffer inflow. Carbohydrate (fiber, starch, or glucose) will be manually fed at 2-h intervals (to maintain near steady-state conditions). Buffer will be infused continuously and will include N sources (trypticase peptides, ammonia, urea), minerals, and clarified rumen fluid. After the 7-d adaptation period, we will sample fermenter contents and effluent once daily over a 3-d measurement period. We will measure concentration of bacterial protein (g L-1) in fermenter contents by using quantitative PCR against 16S ribosomal DNA as described in Aim 2 (below). The composition of bacterial taxa will be determined with sequencing as we have described previously.Study 2 (Pure culture of bacteria)In order to determine if maintenance is impact by carbohydrate source per se (not shifts in bacterial taxa), we will repeat experiments in study 1 but with a single pure culture. We will use Fibrobacter succinogenes S85, which is one of the few bacteria that can grow on either fiber (cellulose) or glucose.AnalysisFor study 1, we will calculate maintenance using regression and then determine if its value differs across carbohydrate sources. Expressing results on an ATP basis (mol ATP-1 g cell protein-1 h-1), we will determine maintenance as ATP production at zero growth rate. After calculating maintenance, we will formally determine if maintenance differs across carbohydrate sources (glucose, starch, fiber) using ANOVA. We will determine if composition of bacterial taxa, also, differs across energy sources. Using 16S ribosomal DNA sequence data, we will calculate within-sample (α) and between-sample (β) diversity using QIIME and procedures we have established, then compare values of these diversity metrics across energy sources using ANOVA. For study 2, experiments for the pure culture will be designed, analyzed, and interpreted similarly, but starch will not be included as a treatment, and no sequence data will be analyzed.Aim 2.Determine how much ATP that mixed rumen microbes expend on glycogen synthesis in vivo.Study 1 (Flows of microbial glycogen and protein)Ruminally-cannulated cows (n = 8) in late lactation will be fed a corn-silage based ration in two equal meals. Following a 14-d adaptation period, we will determine flow of microbial glycogen and protein over a 4-d measurement period. To determine these flows, we will measure 1) total digesta flow (kg/d) using the triple marker technique and omasal sampling, 2) concentration of microbes within digesta (kg/kg) using qPCR, and 3) concentration of glycogen and protein within microbes (kg/kg) using chemical analysis. To determine the concentration of protozoa and bacteria in omasal digesta, we will use small ribosomal subunit DNA (16S and 18S rDNA) as a microbial marker. To determine the concentration of glycogen in isolated bacteria and protozoa, we will use glucose released from glycogen after enzymatic hydrolysis.Study 2 (Dynamics and source carbohydrate for glycogen deposition)We will use n = 4 ruminally-cannulated cows managed as in study 1. Following 14 d of adaptation, we will pulse dose 13Clabeled carbohydrate (glucose or maize cellulose in amounts below) via the cannula during the morning feeding (n = 4 animals per carbohydrate). At 4-h intervals over a 48-h measurement period, we will sample rumen contents, isolate groups as described above, and measure 13C-enrichment of glycogen with isotope ratio mass spectrometry. For study 1, we will calculate ATP required to synthesize microbial glycogen and protein flowing through the omasum. We compare these values (ATP required for glycogen vs. protein) to determine if glycogen is indeed a major sink for ATP. First, we will calculate omasal flows of glycogen and protein, then calculate total ATP required for synthesis glycogen and protein. We will do calculations for bacteria and protozoa separately, and then formally compare values for these two microbial groups using ANOVA. For study 2, we will determine the fraction of carbohydrate deposited into glycogen (mol/mol) over time from 1) total glycogen, 2) 13C-enrichment of glycogen, and 3) 13C dosed. We will compare the fraction deposited across microbial group (protozoa, bacteria) and times after feeding using ANOVA.Aim 3.Determine the ATP yield from the major fermentation pathways of glucose (hexose)Study 1 (Ion pumps Rnf and Ech)We will determine if Ech and Rnf have activity in 1) pure cultures of bacteria and 2) mixed bacteria isolated from the rumen. We will include bacteria that encode and are expected to have activity for 1) both Rnf and Ech or 2) Rnf only. These bacteria are selected based on genome searches. In additional experiments, mixed bacteria will be isolated from rumen fluid as described for Aim 2. To assay for activity of Rnf, we will first prepare cell membranes by 1) disrupting cells in a French pressure cell press then 2) pelleting membranes by ultracentrifugation. All components for the assay (e.g., membranes, buffer, redox cofactors) will be added to a cuvette. Rnf activity will be monitored spectroscopically by reduction of the oxidized NAD (NADox) in the presence of reduced ferredoxin (Fdred). To assay for activity of Ech, we will follow a two-step approach. First, we will determine if bacteria produce hydrogen from reduced ferredoxin. Second, we will determine if bacteria pump protons in response to adding reduced ferredoxin.Study 2 (Glycolytic enzyme Pfp)Using similar approaches to study 1, we will determine if bacteria and protozoa have an unconventional glycolytic enzyme, Pfp, which spares ATP during glycolysis. For bacteria, we will also determine if bacteria have the proton pump HppA, which generates pyrophosphate needed by the enzyme Pfp. For pure cultures of bacteria, we will include species that encode and are expected to have activity of Pfp.As controls, we will include bacteria that do not encode Pfp.Mixed bacteria and protozoa will be isolated from rumen fluid as described for Aim 2. To assay for activity of Pfp, we will prepare cytoplasmic extract by a similar method as in study 1 for membranes, but we will use the supernatant (not pellet) resulting from ultracentrifugation. To determine the kinetics of Pfp vs. Pfk, we will use enzyme derived from Pr. brevis GA33, a bacterium known to have activity of these enzymes. We will produce the enzyme recombinantly in E. coli (using an Invitrogen pET TOPO cloning and expression kit). To assay for activity for the HppA proton pump, which forms pyrophosphate, we will prepare inverted membrane vesicles also using P. brevis GA33.We will determine if protons are pumped into the vesicles after adding pyrophosphate.AnalysisFor study 1, we will determine if activity of Rnf or Ech for each bacterium is different from 0 using ANOVA. For Ech, this will in fact involve examining if two different activities (hydrogen production, proton pumping) are different from 0. For study 2, we will analyze Pfp activity using methods for study 1. For recombinantly produced Pfp and Pfk, we will compare parameters Km, Vmax, and Ki using t-tests. Further, we will estimate the activity of Pfp and Pfk using these parameters, the Michaelis-Menten equation, and plugging in concentrations of substrates and products. As in study 1, all experiments will be repeated at least three times.

Progress 04/01/24 to 03/31/25

Outputs
Target Audience:The project director (PD) works closely with collaborating scientists, undergraduate students, graduate students, dairy nutrition specialists, and dairy producers. Changes/Problems: Nothing Reported What opportunities for training and professional development has the project provided?The PD instructed two PhD students and several undergraduate students in laboratory techniques during completion of experiments. Specifically, one PhD student and several undergraduates learned how to perform experiments with continuous culture fermentors. Fermentors are widely used in animal nutrition and other fields, making this an important skill to learn. Additionally, a second PhD student learned how to perform the aforementioned microbiological experiments with steers. This student secured a tenure-track faculty position, showing the importance of this training. How have the results been disseminated to communities of interest?The PD has disseminated results to dairy nutritionists, feed companies, and startups. Over the reporting period, five groups have visited his lab to see operation of the continuous culture system used to carry out Aim 1. This system acts as a conversation piece for sharing results of the entire project. One additional group visited his lab to learn techniques with rumen protozoa used in Aim 2. In addition to in person visits, the PD has had Zoom calls with several nutritionists and startups. What do you plan to do during the next reporting period to accomplish the goals?We plan to complete experiments of Aim 2 over the next reporting period. These experiments will involve studying glycogen storage in microbes as in the current reporting period, but using isotopically-labeled glucose to trace storage in detail. These experiments will give more insight into how and when glycogen is stored in rumen microbes, help improve efficiency of microbial growth, and help improve formulation of rations for cattle.

Impacts
What was accomplished under these goals? Our project addresses the problem that microbes in the rumen (cow forestomach) grow inefficiently. If efficiency could be improved, it would increase the amount of protein digested by the cow. Overall, our project has led to a change in knowledge of microbial efficiency and will help improve efficiency of livestock production at large. In Aim 1, we found that rumen microbes grow with similar efficiency on two different carbohydrates (glucose and cellulose). It had been thought that microbes grow more efficiently on cellulose vs. glucose, but our controlled experiments with continuous culture showed no clear difference. In detail, we inoculated a system of 8 fermentors with rumen fluid, fed them glucose or cellulose (30 mmol hexose L-1 d-1), and maintained them at a range of dilution rates (2 to 12% h-1). We then measured digestion of carbohydrates and output of microbes and fermentation products. We found that distinct communities of bacteria grew in fermentors fed glucose vs. cellulose, and they formed different profiles of fermentation products. Despite these differences, these communities grew with similar efficiency. Similar efficiency was observed regardless of the measure of efficiency used [g dry cells (mol hexose fermented)-1, g cell dry matter (mol ATP)-1, g cell N (mol hexose fermented)-1, or g cell N (mol ATP)-1]. These results suggest that source of carbohydrate may not be an important factor in determining efficiency of microbial growth in the rumen. It will help the search for other factors that affect microbial growth and formulate better rations for cattle. In Aim 2, we found that rumen protozoa synthesize more glycogen (carbohydrate) than do rumen bacteria. When microbes synthesize glycogen, it diverts energy from growth and can thus depress growth efficiency. It was thought that protozoa store more carbohydrate based on in vitro studies, and our current in vivo experiment confirm it. In detail, 8 Angus-cross and four American Aberdeen steers were fed either a forage-based backgrounding diet or a grain-rich finishing diet in a crossover design. The finishing diet reduced dry matter and fiber intake, lowered ruminal pH, and increased microbial protein synthesis efficiency by 46%, while also enhancing glycogen accumulation in ruminal protozoa. Notably, protozoa contributed more nitrogen flow to the omasum under the finishing diet and stored more glycogen per unit of protein and mass than bacteria. Our results suggest that glycogen synthesis is important in the metabolism of rumen protozoa, and this may depress their efficiency of growth. This work will also help formulate better rations for cattle. Aim 3 was completed during the previous reporting period, and there are no additional accomplishments to report.

Publications

  • Type: Other Journal Articles Status: Accepted Year Published: 2024 Citation: Hackmann TJ. 2024. The vast landscape of carbohydrate fermentation in prokaryotes. FEMS Microbiol Rev. 2024 Jun 20;48(4):fuae016. doi: 10.1093/femsre/fuae016


Progress 04/01/23 to 03/31/24

Outputs
Target Audience:The project director (PD) works closely with collaborating scientists, undergraduate students, graduate students, dairy nutrition specialists, and dairy producers. Changes/Problems: Nothing Reported What opportunities for training and professional development has the project provided?The PD has instructed a PhD student and undergraduate student in laboratory techniques during completion of experiments. How have the results been disseminated to communities of interest?The PD has phone conversations and meetings with dairy nutrition specialists and producers. What do you plan to do during the next reporting period to accomplish the goals?For Aim 1, we will finish analysis of the experiments recently completed. For Aim 2, we will finish analysis of experiments for study 1, and we will complete experiments for study 2.

Impacts
What was accomplished under these goals? We have made progress in Aim 1 by finishing all experiments. The goal of these experiments was to compare energetic efficiency of rumen bacteria growing on glucose vs. cellulose. Preliminary analysis of our results shows that microbes grow more efficiently on the latter. We inoculated a system of 8 single-flow, continuous culture fermenters with rumen fluid, fed them glucose or cellulose (46 mmol hexose d-1), and maintained them at a range of dilution rates (2 to 12% h-1). We then measured digestion of carbohydrates and output of microbes and fermentation products. Our experiments followed a completely randomized design replicated over 3 periods. We found that microbes grew more efficiently [g cells (mol hexose digested)-1] when fed cellulose vs. glucose, especially at high dilution rates. We formally analyzed differences in efficiency by fitting a statistical model to estimate maintenance requirements and maximum growth efficiency. This model showed that maximum efficiency was higher when cells were grown on cellulose [185 g cell (mol hexose)-1] vs. glucose [83 g cell (mol hexose)-1]. Maintenance requirements did not differ by carbohydrate, and they averaged 405 (37 SEM) µmol hexose (g cell)-1 h-1. Similar relationships were observed when efficiency was expressed as g cell (mol ATP)-1. These results show that rumen microbes grow more efficiently on cellulose vs. glucose, and this owes to higher maximum growth efficiency, not lower maintenance requirements. These results help explain why microbes grow with variable efficiency in the rumen and will help formulate diets to maximize this efficiency. We have made progress in Aim 2 by finishing all experiments for study 1. The goal of these experiments was to quantify how much microbial glycogen and protein flows from the rumen of cows. We have begun to analyze results and are comparing the relative contributions of protozoa and bacteria. We have also made progress in Aim 2 by completing a set of preliminary experiments for study 2. The goal of these experiments is to measure kinetics of glycogen synthesis by microbes in the rumen. These experiments involve dosing 13C-glucose in the rumen as a tracer, and we have dosed 13C-glucose in batch cultures to determine the most appropriate dose. Aim 3 was finished prior to the current reporting period.

Publications

  • Type: Other Status: Other Year Published: 2023 Citation: Hackmann TJ, Zhang B. 2023. The phenotype and genotype of fermentative prokaryotes Sci Adv. 9:eadg8687. Zhang B, Lingga C, De Groot H, Hackmann TJ. 2023. The oxidoreductase activity of Rnf balances redox cofactors during fermentation of glucose to propionate in Prevotella. Sci Rep. 2023 13:16429. Hackmann TJ. 2024. New biochemical pathways for forming short-chain fatty acids during fermentation in rumen bacteria. JDS Comm. In press.


Progress 04/01/22 to 03/31/23

Outputs
Target Audience:The project director (PD) works closely with collaborating scientists, undergraduate students, graduate students, dairy nutrition specialists, and dairy producers. Changes/Problems: Nothing Reported What opportunities for training and professional development has the project provided?The PD has instructed a PhD student and undergraduate student in laboratory techniques during completion of experiments. How have the results been disseminated to communities of interest?The PD has phone conversations and meetings with dairy nutrition specialists and producers. What do you plan to do during the next reporting period to accomplish the goals?We will finish experiments in Aim 1 using continuous-culture fermenters. We will continue experiments in Aim 2.

Impacts
What was accomplished under these goals? We made progress in Aim 1 by conducting experiments with continuous-culture fermenters. The goal of these experiments is to compare energetic efficiency of rumen bacteria growing on glucose vs. cellulose. We have completed two out of four planned periods with these fermenters. We made progress in Aim 2 by conducting experiments with ruminally-cannulated cows. The goal of these experiments is to measure kinetics of glycogen synthesis by microbes in the rumen. These experiments involve dosing 13C-glucose in the rumen as a tracer, and we have started preliminary experiments to determine the most appropriate dose.

Publications

  • Type: Other Status: Other Year Published: 2022 Citation: Hackmann TJ. 2022. Redefining the coenzyme A transferase superfamily with a large set of manually-annotated proteins. Protein Sci. doi: 10.1002/pro.4277


Progress 04/01/21 to 03/31/22

Outputs
Target Audience:The project director (PD) works closely with collaborating scientists, undergraduate students, graduate students, dairy nutrition specialists, and dairy producers. Changes/Problems: Nothing Reported What opportunities for training and professional development has the project provided?The PD has instructed a PhD student and undergraduate student in laboratory techniques during completion of experiments. How have the results been disseminated to communities of interest?The PD has phone conversations and meetings with dairy nutrition specialists and producers. What do you plan to do during the next reporting period to accomplish the goals?We will finish experiments in Aim 1 using continuous-culture fermenters.

Impacts
What was accomplished under these goals? We made progress in Aim 3 by finding a new step in fermentation that yields ATP. Specifically, we found Rnf forms ATP during fermentations forming propionate. We found this in two abundant bacteria of the rumen (Prevotella brevis and Prevotella ruminicola), which form propionate or succinate (a propionate precursor). To do this, they use the classic succinate-propionate pathway. At first, this pathway appears unbalanced, forming reduced ferredoxin and oxidized NAD in excess. If this continued unabated, fermentation would halt within 1.5 s. We found these bacteria solve this problem by oxidizing ferredoxin and reducing NAD with Rnf. Additionally, Rnf forms ATP by pumping out sodium ions. We demonstrate this using several approaches (growth experiments, genomics, proteomics, enzyme assays). Rnf thus completes the pathway for forming propionate in these two bacteria and forms ATP. Genomic and phenotypic data suggest many bacteria use Rnf similarly. We cataloged fermentation products of >1,400 species of prokaryotes, and nearly 10% carry out a fermentation forming propionate/succinate and acetate. Over 40% of species carrying out this fermentation also have genes for Rnf, which are otherwise uncommon in prokaryotes. These species come from several habitats (gut, aquatic sediments, anaerobic digesters). This work shows Rnf is important to propionate formation in bacteria from the rumen and other habitats. We made progress in Aim 1 by conducting experiments with continuous-culture fermenters. The goal of these experiments is to compare energetic efficiency of rumen bacteria growing on glucose vs. cellulose. We have completed the first of four periods with these fermenters.

Publications


    Progress 04/01/20 to 03/31/21

    Outputs
    Target Audience:The project director (PD) works closely with collaborating scientists, undergraduate students, graduate students, dairy nutrition specialists, and dairy producers. Changes/Problems: Nothing Reported What opportunities for training and professional development has the project provided?The PD has instructed a PhD student and undergraduate student in laboratory techniques during completion of experiments. How have the results been disseminated to communities of interest?The PD has phone conversations and meetings with dairy nutrition specialists and producers. What do you plan to do during the next reporting period to accomplish the goals?We will conduct experiments in Aim 1 using continuous-culture fermenters.

    Impacts
    What was accomplished under these goals? We made progress in Aim 3 by finding a new fermentation pathway that yields ATP. Specifically, we found a pathway for forming acetate and synthesizing ATP that was unknown in fermentative bacteria. We found the bacterium Cutibacterium granulosum formed acetate during fermentation of glucose. It did not use phosphotransacetylase or acetate kinase, enzymes found in nearly all acetate-forming bacteria. Instead, it used a pathway involving two different enzymes. The first enzyme, succinyl-CoA:acetate CoA-transferase (SCACT), forms acetate from acetyl-CoA. The second enzyme, succinyl-CoA synthetase (SCS), synthesizes ATP. We identified the genes encoding these enzymes, and they were homologs of SCACT and SCS genes found in other bacteria. The pathway resembles one described in eukaryotes, but it uses bacterial, not eukaryotic, gene homologs. To find other instances of the pathway, we analyzed sequences of all biochemically-characterized homologs of SCACT and SCS (103 enzymes from 64 publications). Homologs with similar enzymatic activity had similar sequences, enabling a large-scale search for them in genomes. We searched nearly 600 genomes of bacteria known to form acetate, and we found 6% encoded homologs with SCACT and SCS activity. This included >30 species belonging to 5 different phyla, showing a diverse range of bacteria encode the SCACT/SCS pathway. This work suggests the SCACT/SCS pathway is important to forming acetate in many branches of the tree of life.

    Publications

    • Type: Journal Articles Status: Accepted Year Published: 2021 Citation: Zhang B, Lingga C, Bowman C, Hackmann TJ. 2021. A New Pathway for Forming Acetate and Synthesizing ATP during Fermentation in Bacteria. Appl Environ Microbiol doi:10.1128/AEM.02959-20.


    Progress 04/01/19 to 03/31/20

    Outputs
    Target Audience:The target audience of the workshops is graduate students, faculty, and industry consultants. The audience includes both novices (in the basic workshop) and experienced modelers (in the advanced workshop). Changes/Problems:The workshop was held virtually, not in person, due to the COVID pandemic. What opportunities for training and professional development has the project provided?The workshop was attended by graduate students, faculty, and industry consultants. It trained participants in mathematical modeling techniques important to animal nutrition. How have the results been disseminated to communities of interest?All workshop materials (lectures and hands-on exercises) have been made available on public websites. What do you plan to do during the next reporting period to accomplish the goals? Nothing Reported

    Impacts
    What was accomplished under these goals? A workshop was held at the 2020 American Dairy Science Association (ADSA) meeting and attended by 38 participants. Attendance was lower than in previous years, likely because of the virtual format required by the pandemic. The workshop focused on basic modeling topics, including model construction, evaluating model predictions, meta-analysis, and the Dairy NRC model. Lectures and hands-on exercises were made available on public websites.

    Publications