Source: NORTH DAKOTA STATE UNIV submitted to NRP
ACQUISITION OF DYNAMIC MECHANICAL ANALYZER TO UPGRADE RESEARCH INFRASTRUCTURE
Sponsoring Institution
National Institute of Food and Agriculture
Project Status
COMPLETE
Funding Source
Reporting Frequency
Annual
Accession No.
0211108
Grant No.
2007-35504-18294
Cumulative Award Amt.
(N/A)
Proposal No.
2007-02175
Multistate No.
(N/A)
Project Start Date
Sep 1, 2007
Project End Date
Aug 31, 2008
Grant Year
2007
Program Code
[71.2]- (N/A)
Recipient Organization
NORTH DAKOTA STATE UNIV
1310 BOLLEY DR
FARGO,ND 58105-5750
Performing Department
MECHANICAL ENGINEERING
Non Technical Summary
Polymer matrix composite (PMC) materials combine lightweight elements with excellent strength and other desirable thermal and mechanical properties, making them increasingly desirable alternatives to steel, aluminum, and other traditional engineering materials. The polymer resins and fibers used in PMCs are usually derived from petroleum and other nonrenewable resources; however, renewable oils and fibers are proving to be viable alternatives. A unique collaboration has been established at North Dakota State University (NDSU) that combines expertise from the Agricultural & Biosystems Engineering (ABEN) Department in the processing of northern-grown crops with expertise from the Mechanical Engineering and Applied Mechanics (MEAM) Department in the processing of resins and fibers to develop and manufacture PMCs from renewable resources. Funding to purchase a dynamic mechanical analysis (DMA) instrument is requested in this project to ensure that the biobased polymers developed and used to manufacture biobased PMCs by this group will provide the needed thermomechanical functional properties. Acquisition of a DMA instrument will strengthen the biobased materials partnership at NDSU, provide a new educational tool for materials engineering courses taught at NDSU, and allow this group to be more competitive for federal grants.
Animal Health Component
50%
Research Effort Categories
Basic
50%
Applied
50%
Developmental
(N/A)
Classification

Knowledge Area (KA)Subject of Investigation (SOI)Field of Science (FOS)Percent
40472992020100%
Goals / Objectives
A North Dakota State University (NDSU) multidisciplinary group is seeking to upgrade its research capabilities in order to develop and improve the performance of polymer composite materials (PMCs) created from biobased resins and natural fibers. The objective of this project is to purchase a dynamic mechanical analysis (DMA) instrument because of its ability to perform highly sensitive, dynamic characterization of material properties over a wide temperature range. The acquisition of a DMA will ensure that the biobased polymers and PMCs developed by this group will provide the needed functional properties, provide a valuable educational tool for students in the characterization of biobased materials, and enable this group to compete for federal grants. Specifically, a TA Instruments Q800 DMA is to be purchased through this project and is capable of performing the necessary analysis of neat polymer resin samples, fibers, and PMC samples.
Project Methods
A Dynamic Mechanical Analysis (DMA) instrument performs a highly sensitive, dynamic characterization of materials over a wide temperature range for relating molecular structure, processing conditions, and product properties. In particular, DMA is used extensively to characterize polymers and polymer matrix composites (PMCs) with highly viscoelastic material properties. Specifically for the research initiatives developed by the biobased research group at North Dakota State University (NDSU), the proposed DMA instrument will be used for the following measurements and data collected will be compared against properties commercially available synthetic polymers and PMCs: 1) Glass transition (Tg) or alpha relaxation of the biobased polymers and PMCs developed using a scanning temperature mode. 2) Variation of glass transition in biobased polymers and PMCs developed using a frequency sweep mode. 3) Any secondary transitions in the biobased polymers developed which arise from side group motion with some cooperative vibrations for the main chain as well as internal rotation within a side group. 4) Stiffness of the biobased polymers and PMCs developed and modulus determination using a controlled force/strain rate oscillating mode. 5) Evaluation of the linear viscoelastic range (LVR) of the biobased polymers and PMCs developed using the multi-stress/strain mode. 6) Damping properties of the biobased polymers and PMCs developed by measuring the time lag in the displacement compared to the applied force. The instrument to be procured is the TA Instruments Q800 DMA. The following description is a synopsis of the capabilities described by TA Instruments: Viscoelastic measurements can be achieved on materials over a range of 1000 Pa to 1000 GPa, frequency range of 0.01 to 200 Hz, force range of 0.0001 to 18 Newtons, and amplitude range of 0.5 to 10,000 microns. Resolution is 1 nanometer over the 25 mm drive shaft travel using a linear optical encoder. The temperature range is -150 to 600oC, with the lower end of this range made possible through cooled gaseous nitrogen using the gas cooling accessory with auto-fill capability. The DMA includes a 35 mm dual cantilever bending fixture with digital calipers, steel standards, and torque meter. It also includes a touch control color screen at the module, automated furnace movement, and easy clamping accessibility. Software permits time-temperature superposition, complete experimental control of thermal modules, comprehensive data analysis (Universal Analysis 2000). It includes help menus with diagnostics and multimedia support and is compatible with PC operating on Windows XP. Installation in accordance with an ISO 9000 procedure and training will be provided.

Progress 09/01/07 to 08/31/08

Outputs
OUTPUTS: Funding to purchase a dynamic mechanical analyzer (DMA) instrument was acquired through the NRI Competitive Equipment Grant program. The purchase of this equipment directly impacted the multidisciplinary group of faculty and students (3 faculty and 4 graduate students) involved at North Dakota State University (NDSU) in the development of biobased polymers and the manufacture of biobased polymer matrix composites (PMCs). Acquisition of a DMA instrument has strengthened this biobased materials partnership at NDSU, provided a new educational tool for materials engineering courses taught at NDSU, and has allowed this group to be more competitive for federal grants. Specifically, a TA Instruments Q800 DMA was purchased with this grant and the matching funds that were provided by NDSU. This instrument is a research quality DMA that provides viscoelastic measurements on materials from 1000 Pa to 1000 GPa. The temperature and frequency range of operation are (-150 to 600 deg C) and (0.01 to 200 Hz) respectively. The force range is 0.0001 to 18 Newtons. The amplitude range is 0.5 to 10,000 microns with resolution to 1 nanometer over entire the 25mm of drive shaft travel using a linear optical encoder. The Q800 provides ultra sensitive force measurements down to 0.0001 Newtons, which is ideal for films, fibers, and other materials with low stiffness. PARTICIPANTS: The primary investigator, Dr. Chad Ulven, has gone through extensive training with the equipment purchased (Q800 DMA) along with three graduate students at NDSU (Michael Fuqua, Judith Espinoza Perez, and Kimberly Kramer). Each has spent a considerable amount of time using the equipment for various projects already. In addition to the personnel trained at NDSU to use the equipment, Drs. Dennis Wiesenborn (Co-PI) and Scott Pryor (Faculty Collaborator) and their research staff (Dr. Darrin Haagenson) and student (Wajira Asanga Manamperi) have benefitted from the results obtained to-date. TARGET AUDIENCES: The DMA purchased was demonstrated in the Polymer Engineering course (ME 473/673) taught by Dr. Chad Ulven (PI) in the Mechanical Engineering Department at NDSU in the spring of 2008. The equipment was demonstrated to several undergraduate (25) and graduate students (5) enrolled in the class as a means to evaluate the thermomechanical properties of a variety of thermoplastics. PROJECT MODIFICATIONS: Not relevant to this project.

Impacts
Upon installation, the Q800 DMA was initially used to perform analysis on natural fiber reinforced polypropylene (PP) biocomposites. Using the DMA, variations in both the glass transition temperature (Tg) and the crystallinity change of fiber reinforced specimens was determined. The purpose was to examine the effect that micro-natural fibers derived from dried distiller grains with solubles (DDGS), a corn ethanol by-product, had in PP when modified with various chemical compatibilizers. The Q800 DMA was operated at a frequency of 1 Hz, an amplitude of 20 microns, and a ramp of 3 deg C per min. As PP has a Tg less then ambient room, the liquid nitrogen bulk tank attached to the unit, was employed. Samples were yielded by a composite blending process and a secondary injection molding. Using the DMA, analysis of the alpha-transition of the tan delta curve of the samples was made, corresponding to the Tg of the material as well as the crystallinity change in the specimens. The addition of DDGS was found to decrease the Tg of the neat PP slightly. This indicates that DDGS fibers are being introduced between the polymer chains, increasing the spacing and free volume of the PP. This provides an improvement in damage tolerance within the material in addition to the improvement of strength and stiffness. Several more studies on the DMA such as the one described here are planned for the next few years as the group's efforts to obtain more research funding have been successful as a result of equipment and seed grants like this one.

Publications

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