Source: UNIV OF MASSACHUSETTS submitted to NRP
DEVELOPMENT OF METHODS TO CONTROL LIPID OXIDATION, WATER-HOLDING CAPACITY AND TEXTURE IN MUSCLE FOODS, ESPECIALLY SEAFOOD.
Sponsoring Institution
National Institute of Food and Agriculture
Project Status
COMPLETE
Funding Source
Reporting Frequency
Annual
Accession No.
0209173
Grant No.
(N/A)
Cumulative Award Amt.
(N/A)
Proposal No.
(N/A)
Multistate No.
(N/A)
Project Start Date
Oct 1, 2006
Project End Date
Sep 30, 2010
Grant Year
(N/A)
Program Code
[(N/A)]- (N/A)
Recipient Organization
UNIV OF MASSACHUSETTS
(N/A)
AMHERST,MA 01003
Performing Department
FOOD SCIENCE
Non Technical Summary
Improvising the value of muscle foods can be achieved by maximizing water-holding during processing, storage, and cooking while controlling texture and minimizing lipid oxidation. This research project will address these problems by inactivating oxidation substrates and oxidants and modifying the subcellular structures of the muscle.
Animal Health Component
25%
Research Effort Categories
Basic
75%
Applied
25%
Developmental
(N/A)
Classification

Knowledge Area (KA)Subject of Investigation (SOI)Field of Science (FOS)Percent
5010810100050%
5020810100050%
Goals / Objectives
The overall objective of this work will be to enhance the value of muscle foods, especially sea foods, by improving water-holding capacity, optimizing texture and controlling lipid oxidation. To do this a deep understanding of the major components of the muscle tissue, water, proteins, and lipids is required. Out laboratory has made major inroads in these areas, some of which are now being put into commercial practice. This project will continue this work. Evaluation will be made of the components that are the primary contributors to lipid oxidation in muscle foods. In particular we shall compare heme proteins, other iron proteins and low molecular weight complexed iron. The identified pro-oxidants will be evaluated in isolated membrane systems and in washed and unwashed muscle tissue. Muscles with both high and low content of mitochondria will be examined. To date our membrane work has involved primarily the sarcoplasma particulum, but there is evidence mitochondria also contribute to the oxidation. Control of moisture content of muscle foods is a primary factor in economic yield and quality attributes; a high-water holding capacity (WHC) is desirable. Water-holding capacity is controlled by the structural arrangement of the myofibrillar/cytoskeletal proteins. Injection technology can be used to modify the subcellular muscle structures to allow significant improvements in water-holding capacity of fresh, frozen and/cooked muscle tissue. Improvements in the water holding capacity will be achieved by learning more about the structural rearrangements of the myofibrillar/cytoskeletal proteins as affected by environmental conditions. Important commercial fish are subject to a unique stress, the breakdown of trimethylamine oxide (TMAO) to formaldehyde. When formaldehyde is produced in too high a concentration, the tissue becomes tough and holds water poorly. Our objective is to understand the causes of this effect of formaldehyde and to develop ways of preventing it.
Project Methods
Experiments to inhibit lipid oxidation have involved trying different antioxidants. Our approach is unique in that we determine the fraction of the muscle tissue with which the antioxidant is associated, such as the oil fraction, the lipids of the cellular membranes, the proteins or the aqueous phase. In addition, we shall try to identify the primary pro-oxidants and determine the conditions that are useful in inhibiting their activity. We shall also modify the susceptibility of the most sensitive lipids, those of the membranes, by changing the structure of the membranes. Experimental work justifying all these approaches has been obtained. Our goal with proteins is to evaluate the structural constraints of the myofibrillar and cytoskeletal proteins on water holding-capacity and texture in muscle foods. This will be done by selective solubilization in homogenized, minced and intact muscle tissue. Adjustments to intact muscle tissue will be made by injection techniques. The injection techniques use procedures that do not require phosphates but use protein isolates prepared from low value raw materials from the same species. These concepts are based on work we have done in developing what we have termed the possible solubility inhibiting polypeptides by examining the physical and functional properties of muscle tissue as these protein are selectively solubilized and in some cases removed from the tissue. The selective solubilization is done by modifying the pH and the ionic strength of the aqueous phase of the muscle tissue. A special case involves the role of the formaldehyde produced enzymically from TMAO. This compound reacts with muscle protein to make them highly insoluble and leads to poor-water holding capacity and texture. Although often considered to be caused by cross-linking of the proteins, most experimental evidence including ours shows that this is not the case. We shall take a new approach in the evaluation of the role of formaldehyde by determining whether it functions to modify the possible solubility inhibiting polypeptides of the muscle tissue.

Progress 10/01/06 to 09/30/10

Outputs
OUTPUTS: Acidification of meat can improve texture however it also increases susceptibility to lipid oxidation. The effect of injection and marination of citric acid to acidify and sodium carbonate or sodium tri-polyphosphate to increase pH of beef on tenderness, microstructure and oxidative stability was determined. Water-holding capacity and tenderness of beef semitendinosus muscle increased significantly at pH 3.52 upon addition of citric acid and returned to the level of untreated sample after pH was increased (pH = 5.26) by sodium tri-polyphosphate. The microstructure of the muscle was lost upon acidification but reformed upon increasing muscle pH. Lipid oxidation was inhibited in cooked beef blocks and ground muscle acidified with citric acid. Lipid oxidation was also inhibited in citric acid acidified beef that was re-adjustment to pH values equal to or greater than the raw beef muscle with sodium tri-polyphosphate or sodium carbonate. In addition, citric acid that was adjusted to the pH of the raw beef so that it did not alter the pH of the beef also inhibited lipid oxidation. These results indicate that citric acid and not sodium tri-polyphosphate or pH adjustment was responsible for inhibiting lipid oxidation in beef. These results suggest that the best acid marination technique for beef would be citric acid since it is effective at both improving texture and inhibiting lipid oxidation. PARTICIPANTS: Herbert O. Hultin Eric A. Decker Shuming Ke Yan Huang TARGET AUDIENCES: Food and Meat Processing Industry PROJECT MODIFICATIONS: Dr. Decker has replaced Dr. Hutlin as lead P.I.

Impacts
This research provides the basis of a new technology that can both improve beef tenderness and inhibit lipid oxidation. This would allow meat processors to utilize low value meat cuts in high value processed foods.

Publications

  • Ke, S.; Huang, Y.; Decker, E.A. and Hultin, H.O. 2008. Impact of Citric Acid on the Tenderness, Microstructure and Oxidative Stability of Beef Muscle. Meat Science (submitted).


Progress 10/01/06 to 09/30/07

Outputs
During the extraction of muscle to produce protein isolates by acid or alkali solubilization, membranes are exposed to abnormally low or high pH. Low but not high pH treatment induces rapid oxidation of membrane phospholipids in the presence of hemoglobin. The goal of this research work was to study the oxidative stability of microsomes under the conditions met during acid solubilization. Isolated microsomes from cod muscle were used as a model system. At pH 5.3 or lower, 99% of isolated cod membranes sedimented at low centrifugation speeds. Isolated membranes that were exposed to pH 3.0 were less susceptible to hemoglobin-mediated lipid oxidation. Cod hemoglobin exposed to pH 3 was rendered less pro-oxidative than the untreated cod hemoglobin. However, when microsomes and hemoglobin were together exposed to low pH, oxidation was promoted. Citric acid and calcium chloride, as well as cytsol isolated from cod muscle, were able to inhibit lipid oxidation of microsomal suspensions.

Impacts
Utilization of low pH treatments could inhibit the development of rancidity of fish muscle by protecting cell membranes and inactivating prooxidants. This technique could be used to increase the value and utilization of high fat fish prone to oxidative randicity.

Publications

  • Vareltzis P, Hultin HO Effect of low pH on the susceptibility of isolated cod (Gadus morhua) microsomes to lipid oxidation JOURNAL OF AGRICULTURAL AND FOOD CHEMISTRY 55 (24): 9859-9867 NOV 28 2007