Source: NITRICITY INC. submitted to
HEAT INTEGRATION OF PLASMA REACTORS FOR ELECTRIFIED FERTILIZER PRODUCTION
Sponsoring Institution
National Institute of Food and Agriculture
Project Status
ACTIVE
Funding Source
Reporting Frequency
Annual
Accession No.
1029022
Grant No.
2022-39411-38254
Cumulative Award Amt.
$650,000.00
Proposal No.
2022-04366
Multistate No.
(N/A)
Project Start Date
Sep 1, 2022
Project End Date
Aug 31, 2025
Grant Year
2022
Program Code
[8.4]- Air, Water and Soils
Recipient Organization
NITRICITY INC.
6 COMSTOCK CIR APT 418B
STANFORD,CA 943057717
Performing Department
(N/A)
Non Technical Summary
Founded in 2018, Nitricity is electrifying and distributing the production of nitrogen fertilizer. As it is done today, fertilizer production, distribution, and application emits as much as 5-7%/yr of total global GHG emissions. In this USDA NIFA phase II award, Nitricity builds on work from the phase I award to develop an innovative plasma reactor, the heart of Nitricity's process. In the phase I award, Nitricity improved the efficiency of the reactor and demonstrated the fundamentals of operation. Phase II will focus on improving the energy efficiency further, scaling up the reactor, and applying the principle of heat recovery to improve the overall process. Increasing the scale is important. Through conversations with farmers and fertilizer producers it is clear that the fastest way to reducing the environmental impact of fertilizer is by scaling the Nitricity process from the field level to a community or co-op level as fast as possible. It also allows for economies of scale in the balance of plant. Finally, heat recovery is a general industrial principle were waste heat, which would usually be a liability, is recycled to power another part of the process. Nitricity will apply this concept to our reactor to further improve the energy efficiency of the overall process. Support from this USDA NIFA SBIR phase I grant will support work to reduce environmental impacts from and improve access to fertilizer.
Animal Health Component
(N/A)
Research Effort Categories
Basic
30%
Applied
(N/A)
Developmental
70%
Classification

Knowledge Area (KA)Subject of Investigation (SOI)Field of Science (FOS)Percent
1335210200040%
1335210201060%
Knowledge Area
133 - Pollution Prevention and Mitigation;

Subject Of Investigation
5210 - Fertilizers;

Field Of Science
2010 - Physics; 2000 - Chemistry;
Goals / Objectives
Nitricity Inc. is developing a novel fertilizer production system to turn air, water, and electricity into nitrate based fertilizers. We use a plasma reactor to fix nitrogen into nitric oxide and then absorb this into water to form nitric acid and other nitrate based fertilizers. This grant will build on our phase I work to scale up the reactor and improve heat management and recovery in the reactor. In our commercialization analysis, we identified increased scale as a critical path item for bringing our tech to market. It will allow us to realize economies of scale on the balance of plant and better respond to the customer's needs. In our technical process analysis we found that heat recovery is a pathway to dramatically reduce the total energy consumption of our process. Most of the energy that goes into our reactor is released as high grade heat. Recovering this energy will allow us to offset some electricity use and pumping energy. Our main technical objectives are:(O1) Design and build prototype 15 kW reactor(s) capable of 20 kWh/lb NWe will design and build a prototype reactor capable of fixing nitrogen at a cost of 20 kWh/lbN or less at a power level of 15 kW or more. We anticipate that the results from phase I will allow us to scale(O2) Design and implement heat recovery to the reactor from O1, perform a multivariable sweep to understand the heat transfer.We will use CAD software and measurement of reactor temperature profile to design a heat recovery system, likely including element from fire-tube boilers and shell and tube heat exchangers. The key deliverable will be a physical reactor prototype ready to test for objective 3. We will then explore the parameter space of this reactor, with variables like flow, pressure, power, and cooling water flow rate.(O3) Achieve 80% thermal efficiency of the heat recovery, produce steam of at least 150 psigWe will recover 80% of input energy, defined as the enthalpy of steam divided by the energy input to the reactor. We will do this in the form of high pressure (150 psig) steam. We have identified this as a reasonable input to a heat recovery cycle or steam driven turbomachinery.
Project Methods
Our experimental methods will include:Design of Experiments to explore large multivariable parameter spacesstatistical analysis of that data to find optimal operating points and guide future experimentsInfrared spectroscopy to analyze gas phase productsopticalemission spectroscopy to analyze plasma propertiesPower meters and specialized electronics to measure input powerWe will evaluate the efficiency of our reactor in terms of pounds of nitrogen oxidized per kilowatt hour of energyconsumed by the reactor. To measure the Nitrogen oxidized, we will use FTIR or similar techniques to measure the composition of the outlet gas. To measure the power consumed, we will use power meters or dedicated diagnostics on the power equipment. To measure energy recovered in the boiler, we will measure the flow rate, temperature, and pressure of the streams entering and leaving the boiler. We will use steam table to look up the enthalpy of water at those states.Ultimately, we will evaluate the success of the project on the demonstration of a successful pilot facility that brings in customers and allows us to become a successful business. To do this, we will continue to reach out to customers and develop relationships with farmers, distributors, and industrial players in agriculture.

Progress 09/01/23 to 08/31/24

Outputs
Target Audience:Our target audience is company stakeholders including employees, investors, potential customers, and collaborators. Changes/Problems:The major challenge we faced was permitting and construction timelines for our larger test reactor. We have alleviated these problems by requesting and recieving an extension for the grant timeline as well as engaging with our GC to help move the permitting timelines along. What opportunities for training and professional development has the project provided?This project has created an opportunity for our thermal design engineer to improve his skills in 3D simulations as well as the set up of a clioud cimputing system. How have the results been disseminated to communities of interest? Nothing Reported What do you plan to do during the next reporting period to accomplish the goals?As noted in the request for extension: The testing for a heat recovery solution has not been completed. This effort has not been completed due to ongoing business activities using the 30-kW. This effort is planned to switch to the 100-kW but is being held up by permitting challenges. Scaling from the small scale to large scale system has been held up by the construction timeline, due to permitting delays. The engineering development on the 100-kW system is more complex than initially anticipated and drove the schedule to the right. The team has brought on licensed contractors to operate the systems and improved safety requirements.

Impacts
What was accomplished under these goals? As noted in our requrest for an extension, with an update for objective 2: Objective 1: Improvements to the 30kW system will be incorporated based on these results by adding an oxygen membrane to the inlet gas to enrich the stream with oxygen in a more efficient way. This effort has not been completed due to ongoing business activities using the 30kW. This effort is planned to switch to the 100-kW but is being held up by permitting challenges. We ahve demonstrated the efficiency improvement with compressed oxygen, but not implemented with an oxygne seperating membrane. Objective 2: The heat recovery tests are to be performed in 2024 and test plan schematics will be reported in the Final technical report. The design of the heat exchanger came in lighter than anticipated and due to permitting challenges, labor spending was limited while the system got approval to run. Update: The heat exchanger was tested fot both heat recovery in the small scale system (6kW) and for basic function in the larger scale system (30kW) In both cases, the heat exchanger performed as expected. Objective 3: A heat recovery design will be implemented and tested on the 30-kW system. Objective 3 has not started. Testing is planned in early 2024 to determine efficiency of heat recovery design. Results will be reported in the Final Report due at the end of the Phase II grant period.

Publications


    Progress 09/01/22 to 08/31/23

    Outputs
    Target Audience:Our target audience for this research are internal customers as well as investors and prospective partners. Internal customers include the process development team that needs to make design choices for our product based on the data collected here. Investors and prospective customers include major food companies and venture capitalists who use the data to assess our readiness. Changes/Problems: Nothing Reported What opportunities for training and professional development has the project provided?This project has provided our thermal design engineer with experiencein modelling as well as setting up computer networks. This was achieved by one on one mentorring by project PI Dr. Jay Schwalbe as well as frequent interaction with vendors and technical support. How have the results been disseminated to communities of interest? Nothing Reported What do you plan to do during the next reporting period to accomplish the goals?To complete O1: - implement proposed efficiency improvements from single reactor level to the complete 30kW process To complete O2: - We anticipate that we will receive our first test article at the end of 2023. We will validate if this meets our expectations and begin design for the final test article to complete objective 3. To complete O3: - completing objective 3 will entail taking the lessons from objective one and completing testing.

    Impacts
    What was accomplished under these goals? Nitricity is developing a process to reduce the climate and environmental impact of Nitrogen fertilizer. Our process utilizes a plasma reactor to transform nitrogen and oxygen in the air into valuable nitrate-based fertilizers. Because plasma is generated using electricity and none of our inputs are fossil fuels, we can readily integrate with renewable energy sources and fully reduce the carbon dioxide emissions associated with fertilizer production. In this project, we are working to improve the overall energy efficiency of our process by using heat integration. Most of the energylosses in our system come in the form of high-grade heat in the reactor, so it is a prime candidate for heat recovery. If successful, this initiative will make our process a cost competitive way for farmers or farming communities to produce fertilizer using only air, water, and renewable energy. This will in turn reduce dependence on imports and fossil fuels. We made substantial progress on objective 1 and 2 in the first half of this grant. O1: Nitricity began operation of a 30kW system. We were able to achieve better than the target efficiency on an individual reactor level and will be able to scale this up to the full 30kW as our construction schedule allows. The data collected includes FTIR measurements of reactor output, detailed analysis of the power input, and total system nitrogen fixation. O2: Nitricity performed flow dynamics simulations of the reactor described above for objective 1. We predicted the exit temperature of the reactor based on coolant flows as well as pressure drop in the system. These were observed to be close to the actual values. We also engaged with a manufacturer of heat exchangers to design and fabricate a heat exchanger suitable as a first article to test total heat recovery and aid in the design of the final test article for objective 3. To date, Nitricity has undertaken a major effort to scale up its technology and found new ways to recover high grade heat lost in the reactor. Looking forward to the rest of this grant, we will be able to design and procure heat recovery equipment capable of improving the economics of our process.

    Publications