Source: GROW BIOPLASTICS, LLC submitted to
IMPROVING SUSTAINABILITY AND EFFICIENCY IN HORTICULTURE WITH DEGRADABLE LIGNIN-POLYMER CONTAINERS
Sponsoring Institution
National Institute of Food and Agriculture
Project Status
COMPLETE
Funding Source
Reporting Frequency
Annual
Accession No.
1019655
Grant No.
2019-33610-29801
Cumulative Award Amt.
$106,500.00
Proposal No.
2019-00622
Multistate No.
(N/A)
Project Start Date
Aug 15, 2019
Project End Date
Apr 14, 2022
Grant Year
2020
Program Code
[8.13]- Plant Production and Protection-Engineering
Project Director
Bova, A.
Recipient Organization
GROW BIOPLASTICS, LLC
487 SAM RAY BURN PKWY
LENOIR CITY,TN 377713356
Performing Department
(N/A)
Non Technical Summary
The marketplace adoption of bioplastics over petroleum-based plastics is gaining pace and popularity, in part from increased regulation, but also as a result of grassroots efforts and emerging corporate sustainability, environmental, and human health concerns. Within this material subset exists bio-based, compostable and biodegradable plastics. These materials are often used in agricultural applications such as plastic mulch film, plant containers, seed trays, and many small items like vine clips and twine. In horticulture, the promise of compostable and biodegradable bioplastics carry a massive benefit for plant health and sustainability, but they are plagued by poor durability and high costs - generally 2-3x the price of their petroleum counterparts. The US alone consumes over 5 billion petroleum-based plastic containers each year (750,000 metric tons of plastic), resulting in $3.8 billion in spending, and scalable solutions are needed to address this plastic waste problem.In this proposal, our goal is to investigate the performance of lignin-polymer-based horticultural containers. We will evaluate container durability during automated filling, transplanting, and irrigation processes. We will also focus on potential benefits to plant health measuring plant size, aesthetics, root structure, and soil microbial population and water nutrient content. To test these variables, we are planning to conduct two greenhouse production trials with three container types and 3-4 short-cycle plant species. When commercialized, lignin-polymer containers could be used in commercial greenhouses around the world. Successful implementation of our lignin-based materials into horticulture is a stepping stone to produce a larger portfolio of products addressing the over $12.5 billion in agricultural plastics. Farms and nurseries across the country are highly interested in new biodegradable plastic solutions in the field that have tunable, switchable biodegradation, strengthening this opportunity for sustainable innovation in the US food and agriculture system.
Animal Health Component
75%
Research Effort Categories
Basic
(N/A)
Applied
75%
Developmental
25%
Classification

Knowledge Area (KA)Subject of Investigation (SOI)Field of Science (FOS)Percent
2052122106050%
2052129106050%
Goals / Objectives
ProblemToday, nearly 75 years after the adoption of petroleum containers, the horticulture industry is valued at $90 billion in global market size. The US alone consumes over 5 billion petroleum-based plastic containers each year (750,000 metric tons of plastic), resulting in $3.8 billion in spending. While there are several advantages of using petroleum-based containers, like low cost, good durability, and good manufacturability, there is growing awareness of the downsides, from plastic waste pollution and lack of recyclability to negative impacts on root and plant health. In terms of sustainability, using petroleum as a feedstock leads to greenhouse gas emissions from extraction, refining, and material production and the resulting materials are generally not degradable due to the strong carbon-carbon bond structure of many petroleum-based polymers. In contrast to petroleum-based plastics, bioplastics (plastics produced from renewable resources) are being investigated as an alternative material with potential plant health and biodegradability benefits. The most commonly used bioplastics are polylactic acid (PLA), polyhydroxyalkanoates (PHAs), bio-polyethylene (Bio-PE) and bio-polypropylene (Bio-PP). PLA is the most abundant bioplastic and while naturally brittle, can be modified to have reasonable mechanical properties compared to petroleum plastics. PLA is only degradable in industrial composting conditions and the raw material is expensive, limiting applications in horticulture. PHAs also exhibit reasonable mechanical properties and are readily degradable in soil, but limited availability and high cost prevent widespread adoption. Bio-PP and Bio-PE are created using bio-based feedstocks, such as sugarcane, and have mechanical properties identical to petroleum-based polyethylene and polypropylene but lack biodegradability due to their chemical structure. To mitigate these downsides, researchers are investigating the combination of bioplastics with fillers, additives, and colorants to improve the mechanical properties, lower cost, and improve aesthetics; however, the addition of colorants has shown to decrease biodegradability even at low concentrations, and some additives like carbon black have known human health and environmental effects.Availability and cost are two of the most significant drawbacks for bioplastics today. The global production of PLA, PHAs, Bio-PP, and Bio-PE combined is estimated at 690,000 metric tons and is expected to grow to 2,180,000 metric tons by 2020. In theory, this could satisfy the 750,000 metric ton plastic material demand for horticulture but competition with other markets such as consumer goods and packaging will diminish the quantity of plastic available for horticulture. In addition, the price of these bioplastics today is too high to see more widespread adoption compared to commodity prices for polyethylene and polypropylene.There is an opportunity for a new bio-based material platform to produce a family of low-cost and biodegradable containers with a range of mechanical performance, sustainability, and plant health properties. The existing work to identify new bioplastic formulations for containers in horticulture has not found a material that can match the price, availability, and performance of petroleum-based plastics. The work to date has focused on using PLA or PHAs as the primary polymer and adding fillers, colorants, and other additives to improve performance. Even with increases in availability and decreases in price, poor degradability of materials like PLA are difficult to overcome. In contrast, lignin is a biopolymer produced as a waste product from the paper and biofuel industry at a rate of over 100 million tons per year, is widely available for use as a biorenewable material feedstock, and is very low cost. Lignin can be used as the foundation for a new family of bio-based and biodegradable container materials.Major GoalThe Major Goal of this project is to develop a degradable lignin-polymer horticulture container that can be used in commercial greenhouse operations. In Phase I, our goal is to investigate the performance of lignin-polymer-based horticultural containers. We will evaluate container durability during transplanting, irrigation, and automated processes and plant health, measuring plant size, aesthetics, root structure, and soil conditions. To test these variables, we are planning to conduct two greenhouse production trials with three container materials and 3-4 short-cycle plant species. At the end of Phase I, we will make material recommendations for specific crop types and growing conditions.To accomplish our objectives described below, we are proposing a 3-stage research plan to investigate the effectiveness of lignin-polymers as a material feedstock for horticultural containers, looking specifically at the durability and mechanical properties during and after greenhouse production and the impacts on plant and root health. To do this, we will compare two of our material formulations against polypropylene (PP) as a control throughout the greenhouse production cycle, starting with tests to evaluate durability. These durability tests will subject our containers, and the PP controls, to standard automation, irrigation, transportation, and transplanting processes and evaluate the condition of the containers afterwards. We will evaluate Crush Strength and Wet Strength of containers before and after these processes to characterize the effects of watering and handling on mechanical performance. To study the effects of lignin-bioplastic containers on plant health, we will grow short-cycle greenhouse crops in the various containers in a commercial greenhouse. In order to gather sufficient data, we will carry out these tests using 3-4 different plant varieties, including Calibrachoa, Petunia, Vinca, and Penta, in a standard soil mix, based on recommendations from our greenhouse partners. These are crops with a high tolerance to changes in pH and are in high commercial demand for retailers. With the time permitted by the grant, we will be able to perform two production trials, which will allow us to test these plants multiple times throughout the year and/or select new plants for the trials. To characterize plant health, we will measure plant shoot size, root health (evidence or absence of root circling), plant and flower color, presence or absence of chlorosis/necrosis, water nutrient content, soil microbial health (presence or absence of pathogenic microbes) and the dry weight of roots and plant biomass. To address these challenges, we have the following Objectives for this project:Assess lignin-polymer container durability and performance during automation, irrigation, and transplanting trials during regular greenhouse production operation. In this objective, we will test our containers in a commercial greenhouse environment including automated soil filling equipment, automated seeding and transplanting, and regular irrigation to determine material durability. Evaluate lignin-polymer container mechanical properties after a full greenhouse crop cycle. In this objective, we will work with our greenhouse partners to carry out production trials of 3-4 recommended annual crops, evaluate the condition of the bioplastic containers after the trial, and compare them to the condition of petroleum-based container controls.Evaluate plant health of crops grown in lignin-polymer containers, based on root structure, plant size, color, and soil conditions. In this objective, we will evaluate the growth and health of the plants grown in bioplastic containers compared to petroleum-based container controls to determine if there are benefits from a bioplastic container during product.
Project Methods
The following Methods will be used to evaluate the Objectives mentioned above.Objective 1: Assess lignin-polymer container durability and performance during automation, irrigation, and transplanting trials during regular greenhouse production operationIn this objective, we will compare two formulations of our lignin-polymer blends against polypropylene (PP), a common plastic used for horticulture containers, during automation, irrigation and transplanting. To evaluate these materials, groups of 10 containers will be placed on a tray. We will use standard soil filling equipment with our greenhouse partners to evaluate the performance of our materials. In normal operations, trays of containers are conveyed through these machines to fill them with soil. After filling, we will inspect each container to see if any were crushed or cracked. This will provide us with material scores for Crush Strength. Following filling, we will water each tray and inspect the durability of each pot after they are sufficiently wet, providing scores for Wet Strength. After watering, the trays will be moved to the transplanting area prior to Stage 2. During the transportation step, we will evaluate the durability and usability of these containers for simple tasks like handling and moving.Objective 2: Evaluate lignin-polymer container mechanical properties after a full greenhouse crop cycleWe will work with our partners to carry out production trials with 3-4 recommended crops, including Calibrachoa, Petunia, Vinca, and Penta, in a standard soil mix. After a few weeks, the seedlings for these crops will be ready for transplanting into larger 4.5" containers for greenhouse production. At this stage, we will have 3 container types (lignin-polymer blend 1, lignin-polymer blend 2, and petroleum-based control), 3-4 plant varieties, and 20 replicates for each container/species unit. After each crop is grown to a sufficient size and would be ideally ready to be shipped to a retailer, we will conclude the production trial. At the conclusion of the trial, we will evaluate the integrity and aesthetic quality of the containers compared to new containers and control PP containers. Objective 3: Evaluate plant health of crops grown in lignin-polymer containers, based on root structure, plant size, color, and soil conditions.As mentioned above, we will work with our partners to carry out production trials with 3-4 recommended crops, including Calibrachoa, Petunia, Vinca, and Penta, in a standard soil mix. After each crop is grown to a sufficient size, we will conclude the production trial. At this point, we will separate the plants and soil from the container for follow-on analysis. We will be evaluating the presence or absence of root-circling, plant appearance and health, based on leaf color, presence or absence of chlorosis/necrosis, flower color (if applicable), cell counts of soil microbes, water-use efficiency, nutrient content, and soil pH. We will then separate the plants from the roots and dry them in order to quantify the root, plant, and root-to-plant ratio of biomass. These factors are indicative of plant healthObjectives 2 & 3 will be repeated in a second greenhouse trial. Many of the crops have ideal growing conditions and recommended growing times throughout the year that are useful for commercial production. In an R&D context, plants are often grown throughout the year to observe changes in plant growth and evaluate the effects of new growing practices, new material choices, or new plant breeds. By repeating these experiments, we can see if the time of year and variations in greenhouse operations impact container performance, plant growth, and plant health.SBIR Phase II R&D Plan. Our go/no-go metric for pursuing a Phase II grant to continue development of this technology is that "Lignin-polymer containers demonstrate mechanical properties similar to petroleum-based containers and/or show improvements in plant health." Demonstrating material performance is very important for commercial adoption by large-scale greenhouses. Similarly, improvements in plant health would have significant impacts on the economics of plant sales for both greenhouses and retailers. In Phase II, we will continue to investigate the material formulations from Phase I and if necessary, expand the sample size to include new formulations with: soy-protein or distillers' grain additives to improve plant health and other lignin/polymer combinations to evaluate other mechanical properties. A longer Phase II experiment will also expand the scope of greenhouse crops used to include medium and long-cycle crops. We have a particular interest in nursery containers as this product could be beneficial to large paper companies who plant millions of trees each year to support their business models. A Phase II R&D plan would also include an end-of-life study to evaluate the biodegradability of lignin-polymer containers in different soil types.

Progress 08/15/19 to 04/14/22

Outputs
Target Audience:The original target audiences for this project were US greenhouses, home-improvement retailers, plastic product manufacturers, lignin suppliers, biopolymer suppliers, US regulators, and the general public (especially those concerned with the sustainability of our food and agriculture system). During the project, the target audience of the project expanded to include stakeholders in the fertilizer industry. Without access to manufacturing facilities and facilities to conduct product trials due to COVID-19, we shifted the milestones of the project to focus on material formulation & development and investigate the potential to develop polymer formulations with added nutrients, which could be turned into a self-fertilizing container in the future. Through our project, we wanted US growers and home-improvement retailers to learn how biodegradable and compostable bioplastic materials can be used in their operations to improve the economics and sustainability of their business by reducing the time and money they spend disposing of plastic waste, and improving plant growth and health. For plastic product manufacturers and their supply chain partners, we wanted to share our insights into bioplastic degradation with them so that we can work with these companies to provide better materials for their customers. As part of our supply chain, we wanted lignin and biopolymer suppliers to see our results in this project and work with them to improve future versions of our products. For the fertilizer industry, we wanted to demonstrate the potential for a new class of controlled-release fertilizer materials that do not contribute to microplastic pollution and show that these can be incorporated directly into durable goods like containers. For US regulators, we want to share these results so that US policies and practices are informed by the most recent science. Current regulations restrict the use of biodegradable and compostable materials for certain agricultural and horticultural applications, such as organic certified crops. As we learn more about how bioplastics degrade and how they impact plant health and growth, we want to share these findings with regulators so that US policies reflect this change in knowledge. For the general public, we want to share our findings so they see the US government is funding work to investigate more sustainable materials and practices in our agriculture system, like adopting compostable and biodegradable bioplastics that mitigate the use of single-use petroleum based plastics that are bound for landfills. Changes/Problems:Major changes We experienced significant delays and challenges during the last 2 years due to COVID which forced us to shift focus during Phase I. Without access to manufacturing facilities and facilities to conduct product trials, we shifted gears to focus more on material formulation & development and investigate the potential to develop polymer formulations with added nutrients, which could be turned into a self-fertilizing container in the future. We also engaged with commercial partners to better understand the needs and specifications for this technology. We worked with our Program Leader, Dr. Thomson, to modify our original work plan to reflect these changes and did not have to modify the budget. Project Goals & Modifications to the Work Plan The focus of our original project was to leverage our core technology for lignin-based biopolymers to produce a biodegradable horticultural container and to evaluate the potential of these materials for plant & soil health benefits. We experienced significant delays and challenges during the last 2 years due to COVID which forced us to shift focus during Phase I. While the original work plan was delayed, we continued to receive numerous inbound requests from potential customers inquiring about biodegradable flower pots, the incorporation of slow-release fertilizer technology into biodegradable flower pots, and standalone slow release fertilizer products. These customers includeflower pot manufacturers,commercial growers,fertilizer companies,and industry tradeassociationslike the International Fresh Produce Association. These new customer interactions have validated our product focus but require a modification to our product development needs. As a result, we pivoted our work plan to focus on the development of lignin-based biopolymers with soil nutrient additives. This work specifically examined different nitrogen forms such that fertilizer is released into the soil in a controlled manner through osmotic gradients and as the lignin-biopolymer degrades via microbial activity in the soil or growing medium. This development opens new product lines like biodegradable, self-fertilizing flower pots and slow-release fertilizers that each of the customers above have some interest in. To address these modified goals, we modified our project hypotheses and specific aims. Hypothesis 1: Lignin-based polymers can match or exceed the durability characteristics of petroleum-based plastics in agriculture and horticulture applications. Hypothesis 2: A lignin-polymer matrix can be used to incorporate added nutrients, like nitrogen, and provide a fertilization effect during biodegradation. Hypothesis 3: The rate of nutrient release can be tuned by the polymer formulation. Hypothesis 4: Production of a pelletized lignin-polymer with added nitrogen is the first step toward more complex products, like multi-nutrient fertilizers, self-fertilizing flower pots, and controlled-degradation mulch films. To evaluate these hypotheses, we proposedthe following three Specific Aims: Specific Aim 1: Evaluate compatibility of lignin, biodegradable co-polymers, and nitrogen sources in batch polymer compounding trials using a torque rheometer. Specific Aim 2: Assess the influence of polymer formulations on nutrient release through lysimeter trials. Specific Aim 3: Identify formulations for small-scale production on a twin-screw extruder. This modified effort was carried out in multiple parts in Phase I, through formulation development trials with lignin, biodegradable copolymers, and various nitrogen sources, nutrient release trials to quantify the fertilization effect of these polymers, and small-scale production trials. In the formulation trials, we evaluated the compatibility of biorefinery and paper mill lignins from commercial suppliers, copolymers, and nitrogen sources. We compounded these ingredients using our patented technology into various formulations and then conducted nutrient release studies in a lysimeter to compare release rates to existing controlled release fertilizer products. We used the data from the formulation trials and nutrient release trials to identify the top 3 formulations for small-scale production trials using commercial twin-screw extruders to produce a pelletized fertilizer. These materials were then used in plant growth trials to observe potential plant health and fertilizer performance. What opportunities for training and professional development has the project provided? Nothing Reported How have the results been disseminated to communities of interest?We have been in contact with industry stakeholders throughout our Phase I project and have shared some of the preliminary results on our nutrient release and plant growth trials. In parallel with our Phase I project, we have been communicating with these stakeholders and customers to better understand the specifications that are required for a minimum viable product, such as mechanical properties, manufacturing properties, and nutrient release profiles. We plan to continue these conversations during Phase II and to disseminate more information after we have sufficiently protected our intellectual property. Business Development & Commercialization Since receiving our Phase I award in 2019, we conducted 3 manufacturing trials, evaluated 2 downstream processing methods, and completed 2 plant growth trials. The manufacturing trials produced raw material and provided opportunity for process improvement. We worked with manufacturing partners to produce container prototypes with injection molding and thermoforming. Lastly, we gained insight on the effect of our materials on plant health and growth in 2 plant growth trials (with vinca and violas) where our material served as controlled release fertilizers. This work has maintained and built upon relationships with customers and industry partners with the shared goal to commercialize the mobius lignin-biopolymer technology for horticulture products. In addition to the technical goals of this project, we accomplished several goals through the TABA Program. We employed Larta Inc to perform market research, a patentability assessment, and review our strategy for commercialization. These outcomes support our goal to develop biodegradable polymers for horticulture containers and other durable agricultural products. Furthermore, conversations with key industry stakeholders revealed an opportunity to develop products with added nutrient content, such as self-fertilizing containers. We plan to address these opportunities in our USDA Phase II application and in other projects. What do you plan to do during the next reporting period to accomplish the goals? Nothing Reported

Impacts
What was accomplished under these goals? Specific Aim 1: Evaluate compatibility of lignin, biodegradable co-polymers, and nitrogen sources in batch torque rheometer trials We evaluated the compatibility of lignin and co-polymers with added sources of nitrogen (specifically nitrogen salts). This expands on our previous work formulating and characterizing lignin-polymer composites for durable goods applications. Our approach investigated the addition of several nitrogen compounds over a range of loadings in several lignin-polymer formulations. Several compounded materials were prepared without lignin to understand the role of lignin content on nutrient release kinetics, and similarly, control samples with only lignin polymer, no lignin content, and neat copolymers, and blanks used to understand the role of lignin on plant and root health, and provide a baseline against zero addition of fertilizer and commercial formulations. During the torque rheometer trials, these formulations were compounded in batch conditions producing 50g of material, under various processing conditions, to reflect the input materials. These materials were then pelletized and examined in the lysimeter trials. There were several challenges compounding formulations due to poor mechanical properties, with the final polymer being too brittle for additional characterization tests. This also informed on continuous processing (Aim 3). Formulations with poor mechanical properties fail to meet our commercialization goals targeting durable goods and products with added nitrogen content for the agricultural industry. Additionally, this preliminary work yielded new ideas on how to improve formulation & production with alternative nitrogen sources and additives, as well as processing steps. Specific Aim 2: Assess the influence of polymer formulations on nutrient release through lysimeter trials To test the ability of lignin polymers to control and regulate the release of compounded nutrients, we needed a standard method to evaluate this property. After reviewing the literature, our team identified lysimeters (small columns of sand and soil) as an experimental method for studying this phenomenon. We constructed lysimeters from PVC pipe and performed the necessary control experiments. Promising polymer formulations from Aim 1 were addd to each lysimeter column, a standard quantity applied. Once a week these columns were flushed with 0.01% citric acid solution and the effluent was collected and measured for nitrogen content (total nitrogen, ammonium, and nitrate). 9 weeks of data was collected to establish nutrient release profiles. Commercially available controlled release fertilizers (Vigoro, Osmocote, and Scotts/Miracle-Gro Shake n Feed) were used as positive controls for these experiments. As part of a separate research project, we conducted two plant growth trials with several of these polymer formulations to investigate the effects of lignin-polymer with added nitrogen on plant growth and health. We mention this here as plant health and growth is an indirect measure of nutrient release based on the assumption that the plants with the best growth and health measures benefited from the release of nutrients. In 2021 and 2022, we conducted two plant growth trials with Violas and Vincas, respectively. The results from the nutrient release experiments (in lysimeters) and the plant growth trials have provided great insight on our formulation development efforts. We observed substantially different nutrient release profiles across the polymer formulations, providing evidence that release rates and quantities could be controlled. We hypothesize that the biodegradability of the co-polymers affects the release rate of nutrients in this polymer system. As a result of these tests, we are confident in our ability to create polymer formulations that match specific nutrient release profiles consistent with commercially available fertilizer offerings ( e.g., 3 month, 6 month, and 12 month fertilizers). The viola growth trial also revealed promising results. In an internal greenhouse trial we measured the effects of nitrogen release on growth of violas, a standard horticultural plant. All plants with mobius formulations grew statistically better than plants without added nitrogen, and the formulations with lignin grew as well as a commercial fertilizer. All mobius formulations had flower counts, a measure of plant attractiveness, that met or exceeded commercial fertilizers, and far exceeded plant treatments without nitrogen. Plants treated with mobius formulations devoted more energy to larger roots than compared to the commercial fertilizer, an indication they are searching for more nutrients. This is likely due to the fact that the mobius formulations only contained nitrogen and were missing key plant nutrients that were included in the commercial fertilizers. Plant mass was also measured at the end of the experiment to understand the efficacy in converting released nitrogen into plant mass. A few of the mobius formulations exceeded commercial fertilizers in this metric. In sum, the plant growth trial had promising results and provided many learnings on how to best conduct a plant trial in the future. We plan to conduct additional hydrostatic experiments to measure the baseline nutrient release rates for each polymer in DI water and study nutrient release rates without the effects of supplement mechanisms, such as polymer degradability. Specific Aim 3: Identify formulations for small-scale production on a twin-screw extruder One key advantage to our technology is continuous processing. Other polymer technologies for controlled release fertilizer production, like polyurethanes, are limited to batch production. Continuous processing is particularly advantageous for controlled-release fertilizer applications which predominantly rely on batch production processes. We evaluated the continuous production of our materials with a small subgroup of promising formulations from Aim 1. This continuous production trial used a Leistritz 27mm twin-screw extruder (40:1 L/D), capable of producing material on the order of 20kg/hr. 3 formulations were selected for thisaim, and nearly 100 pounds of these formulations were produced. This provided material for the plant growth trials described in Aim 2. We are continuing to improve and optimize the production of our materials on the twin-screw extruder, recognizing that our technology is a different implementation of polymers compared to traditional prill coating technology. We are also progressing in our commercialization efforts with early partners and customers, detailed in the Business Development & Commercialization section.

Publications


    Progress 08/15/20 to 06/14/21

    Outputs
    Target Audience:While the proposed work has been delayed due to COVID-19, we've continued to receive numerous inbound requests from potential customers inquiring about biodegradable flower pots and slow release fertilizer products, including m-plastic, Summit Plastics, and HC Companies (flower pot manufacturers), Costa Farms, Monrovia, and Altman Plants (commercial growers), Scotts-MiracleGro (fertilizer company), and the Produce Marketing Association (trade organization for produce and floral industries). These new customer interactions have validated our product focus but require a modification to our product development needs. As a result, we are proposing to pivot our work plan to focus on the development of lignin-based biopolymers with added nitrogen to provide fertilization as our materials biodegrade in soil. The development of lignin-polymers with added nutrient content will serve as a subsystem in developing new product lines like biodegradable, self-fertilizing flower pots and slow-release fertilizers. Changes/Problems:We experienced several delays during our Phase I project due to COVID-19, which impacted our R&D operations and access to facilities, and the initial delay for receipt of our USDA Phase I Award. While the proposed work has been delayed, we've continued to receive numerous inbound requests from potential customers inquiring about biodegradable flower pots and slow release fertilizer products, including m-plastic, Summit Plastics, and HC Companies (flower pot manufacturers), Costa Farms, Monrovia, and Altman Plants (commercial growers), Scotts-MiracleGro (fertilizer company), and the Produce Marketing Association (trade organization for produce and floral industries). These new customer interactions have validated our product focus but require a modification to our product development needs. As a result, we are proposing to pivot our work plan to focus on the development of lignin-based biopolymers with added nitrogen to provide fertilization as our materials biodegrade in soil. The development of lignin-polymers with added nutrient content will serve as a subsystem in developing new product lines like biodegradable, self-fertilizing flower pots and slow-release fertilizers. This effort will be carried out in multiple parts in Phase I, through formulation development trials with lignin, biodegradable copolymers, and various nitrogen sources, nutrient release trials to quantify the fertilization effect of these polymers, and small-scale production trials. In the formulation trials, we will evaluate the compatibility of biorefinery and paper mill lignins (UPM, Ingevity, Renmatix), copolymers (PBS, PBAT, PHA), and nitrogen sources (Ammonium Salts, Nitrate Salts, Urea, etc). We will compound these ingredients into various formulations and then conduct nutrient release studies in a lysimeter to compare release rates to existing controlled release fertilizer products. We will then use data from the formulation trials and nutrient release trials to identify the top 3 formulations for small-scale production trials using commercial twin-screw extruders to produce a pelletized plastic. In Phase II, we will investigate these pelletized plastics for use in commercial products, like flower pots, optimize our formulations, and conduct pilots with commercial partners, like Costa Farms. The Revised Phase I work plan will focus on the following hypotheses: Hypothesis 1: Lignin-based polymers can match or exceed the durability characteristics of petroleum-based plastics in agriculture and horticulture applications Hypothesis 2: A lignin-polymer matrix can be used to incorporate added nutrients, like Nitrogen, and provide a fertilization effect during biodegradation Hypothesis 3: The rate of nutrient release can be tuned by the polymer formulation Hypothesis 4: Production of a pelletized lignin-polymer with added nitrogen is the first step toward more complex products, like fertilizers, flower pots, and mulch films To evaluate these hypotheses, we propose the following three Specific Aims: Specific Aim 1: Evaluate compatibility of lignin, biodegradable co-polymers, and nitrogen sources in batch torque rheometer trials Specific Aim 2: Assess the influence of polymer formulations on nutrient release through lysimeter trials Specific Aim 3: Identify formulations for small-scale production on a twin-screw extruder While these changes affect the work plan, we do not anticipate significant changes to our budget and we anticipate completing these objectives under the revised project timeline with a second no-cost extension. What opportunities for training and professional development has the project provided? Nothing Reported How have the results been disseminated to communities of interest? Nothing Reported What do you plan to do during the next reporting period to accomplish the goals?We plan to evaluate the compatability of lignin, biodegradable polymers, and added nitrogen in batch torque rheometer studies as a precursor to fertilizer and/or self-fertilizing horticultural containers. We will study the initial formulations from this evaluation in lysimters to characterize the nitrogen release profile of these materials.

    Impacts
    What was accomplished under these goals? The initial work plan for this project has been revised with a new set of objectives (with approval from our Program Manager). These will be laid out on the next page.

    Publications


      Progress 08/15/19 to 08/14/20

      Outputs
      Target Audience: Nothing Reported Changes/Problems:Due to delays in receiving funds for this project, we have not yet started this project. We are planning to submit a no-cost extension and will begin the project once we receive funds for the project. What opportunities for training and professional development has the project provided? Nothing Reported How have the results been disseminated to communities of interest? Nothing Reported What do you plan to do during the next reporting period to accomplish the goals? Nothing Reported

      Impacts
      What was accomplished under these goals? Due to delays in receiving funds for this project, we have not yet started this project. We are planning to submit a no-cost extension and will begin the project once we receive funds for the project.

      Publications


        Progress 08/15/19 to 04/14/20

        Outputs
        Target Audience: Nothing Reported Changes/Problems:Due to delays in receiving funds for this project, we have not yet started this project. We are planning to submit a no-cost extension and will begin the project once we receive funds for the project. What opportunities for training and professional development has the project provided? Nothing Reported How have the results been disseminated to communities of interest? Nothing Reported What do you plan to do during the next reporting period to accomplish the goals? Nothing Reported

        Impacts
        What was accomplished under these goals? Due to delays in receiving funds for this project, we have not yet started this project. We are planning to submit a no-cost extension and will begin the project once we receive funds for the project.

        Publications